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Volume 31 Issue 1
Jan 2020
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Article Contents
Lili Liang, Cong-Qiang Liu, Xiangkun Zhu, Bryne T. Ngwenya, Zhongliang Wang, Liuting Song, Jin Li. Zinc Isotope Characteristics in the Biogeochemical Cycle as Revealed by Analysis of Suspended Particulate Matter (SPM) in Aha Lake and Hongfeng Lake, Guizhou, China. Journal of Earth Science, 2020, 31(1): 126-140. doi: 10.1007/s12583-017-0957-8
Citation: Lili Liang, Cong-Qiang Liu, Xiangkun Zhu, Bryne T. Ngwenya, Zhongliang Wang, Liuting Song, Jin Li. Zinc Isotope Characteristics in the Biogeochemical Cycle as Revealed by Analysis of Suspended Particulate Matter (SPM) in Aha Lake and Hongfeng Lake, Guizhou, China. Journal of Earth Science, 2020, 31(1): 126-140. doi: 10.1007/s12583-017-0957-8

Zinc Isotope Characteristics in the Biogeochemical Cycle as Revealed by Analysis of Suspended Particulate Matter (SPM) in Aha Lake and Hongfeng Lake, Guizhou, China

doi: 10.1007/s12583-017-0957-8
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  • Corresponding author: Lili Liang; Cong-Qiang Liu
  • Received Date: 15 Jul 2017
  • Accepted Date: 20 Dec 2017
  • Publish Date: 01 Feb 2020
  • Zn isotope is a useful tool for tracing biogeochemical processes as zinc plays important roles in the biogeochemistry of natural systems. However, the Zn isotope composition in the lake ecosystems has not been well characterized. In order to resolve this problem, we investigate the Zn isotope compositions of suspended particulate matter (SPM) and biological samples collected from the Aha Lake and Hongfeng Lake, and their tributaries in summer and winter, aiming to explore the potential of this novel isotope system as a proxy for biogeochemical processes in aqueous environments. Concentration of dissolved Zn ranges from 0.65 to 5.06 μg/L and 0.74 to 12.04 μg/L for Aha Lake and Hongfeng Lake, respectively, while Zn (SPM) ranges from 0.18 to 0.70 mg/g and 0.24 to 0.75 mg/g for Aha Lake and Hongfeng Lake, respectively. The Zn isotope composition in SPM from Aha Lake and its main tributaries ranges from -0.18‰ to 0.27‰ and -0.17‰ to 0.46‰, respectively, and it varies from -0.29‰ to 0.26‰ and -0.04‰ to 0.48‰, respectively in Hongfeng Lake and its main tributaries, displaying a wider range in tributaries than lakes. These results imply that Zn isotope compositions are mainly affected by tributaries inputting into Aha Lake, while adsorption process by algae is the major factor for the Zn isotope composition in Hongfeng Lake, and ZnS precipitation leads to the light Zn isotope composition of SPM in summer. These data and results provide the basic information of the Zn isotope for the lake ecosystem, and promote the application of Zn isotope in biogeochemistry.

     

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