Advanced Search

Indexed by SCI、CA、РЖ、PA、CSA、ZR、etc .

Volume 28 Issue 3
Jun 2017
Turn off MathJax
Article Contents
Xiaoyu Zhang, Zhongqin Li, Nozomu Takeuchi, Feiteng Wang, Shengjie Wang, Xiaoni You, Ping Zhou. Heavy Metal-Polluted Aerosols Collected at a Rural Site, Northwest China. Journal of Earth Science, 2017, 28(3): 535-544.
Citation: Xiaoyu Zhang, Zhongqin Li, Nozomu Takeuchi, Feiteng Wang, Shengjie Wang, Xiaoni You, Ping Zhou. Heavy Metal-Polluted Aerosols Collected at a Rural Site, Northwest China. Journal of Earth Science, 2017, 28(3): 535-544.

Heavy Metal-Polluted Aerosols Collected at a Rural Site, Northwest China

More Information
  • Daily samples of aerosol (n=27) were collected from September 21st to October 4th, 2013 in Fukang (44.17oN, 88.45oE, 475 m a.s.l.), Xinjiang, Northwest China. The enrichment factors (EFc) of selected 49 elements showed that the aerosols had extremely high concentrations of heavy metals, probably indicating their anthropogenic origins. Morphology of individual aerosol particles was determined by scanning electron microscopy and energy-dispersive X-ray microanalysis. Based on morphology and elemental composition, the particles were clustered into three dominant types: (Ⅰ) crustal originated particles: Si/Al-rich particles (36%) and Si/Fe-rich particles (24%); (Ⅱ) mixed source particles; and (Ⅲ) pollution derived particles: Pb-rich particles (10%). The backward trajectories were calculated using the HYSPLIT model, and the results indicated the different anthropogenic sources for heavy metals in Fukang aerosols. Air mass from north was identified as the most polluted source when compared to south and west.

     

  • loading
  • Ayrault, S., Senhou, A., Moskura, M., et al., 2010. Atmospheric Trace Element Concentrations in Total Suspended Particles near Paris, France. Atmospheric Environment, 44(30): 3700-3707. doi: 10.1016/j.atmosenv.2010.06.035
    Barbante, C., Boutron, C., Morel, C., et al., 2003. Seasonal Variations of Heavy Metals in Central Greenland Snow Deposited from 1991 to 1995. Journal of Environmental Monitoring, 5(2): 328-335. doi: 10.1039/b210460a
    Borbon, A., Locoge, N., Veillerot, M., et al., 2002. Characterisation of NMHCs in a French Urban Atmosphere: Overview of the Main Sources. Science of the Total Environment, 292(3): 177-191. doi: 10.1016/s0048-9697(01)01106-8
    Chakrabarty, R. K., Moosmüller, H., Garro, M. A., et al., 2006. Emissions from the Laboratory Combustion of Wildland Fuels: Particle Morphology and Size. Journal of Geophysical Research, 111: D07204. doi: 10.1029/2005jd006659
    Cheng, H. F., Hu, Y. A., 2010. Lead (Pb) Isotopic Fingerprinting and Its Applications in Lead Pollution Studies in China: A Review. Environmental Pollution, 158(5): 1134-1146. doi: 10.1016/j.envpol.2009.12.028
    Cong, Z. Y., Kang, S. C., Liu, X. D., et al., 2007. Elemental Composition of Aerosol in the Nam Co Region, Tibetan Plateau, during Summer Monsoon Season. Atmospheric Environment, 41(6): 1180-1187. doi: 10.1016/j.atmosenv.2006.09.046
    Cong, Z. Y., Kang, S. C., Luo, C. L., et al., 2011. Trace Elements and Lead Isotopic Composition of PM10 in Lhasa, Tibet. Atmospheric Environment, 45(34): 6210-6215. doi: 10.1016/j.atmosenv.2011.07.060
    Cong, Z. Y., Kang, S. C., Zhang, Y. L., et al., 2010. Atmospheric Wet Deposition of Trace Elements to Central Tibetan Plateau. Applied Geochemistry, 25(9): 1415-1421. doi: 10.1016/j.apgeochem.2010.06.011
    Duce, R. A., Hoffman, G. L., Zoller, W. H., 1975. Atmospheric Trace Metals at Remote Northern and Southern Hemisphere Sites: Pollution or Natural?. Science, 187(4171): 59-61. doi: 10.1126/science.187.4171.59
    Fang, M., Zheng, M., Wang, F., et al., 1999. The Long-Range Transport of Aerosols from Northern China to Hong Kong--A Multi-Technique Study. Atmospheric Environment, 33(11): 1803-1817. doi: 10.1016/s1352-2310(98)00318-5
    Ferrari, C. P., Clotteau, T., Thompson, L. G., et al., 2001. Heavy Metals in Ancient Tropical Ice: Initial Results. Atmospheric Environment, 35(33): 5809-5815. doi: 10.1016/s1352-2310(01)00347-8
    Güllü, G. H., Ölmez, I., Aygün, S., et al., 1998. Atmospheric Trace Element Concentrations over the Eastern Mediterranean Sea: Factors Affecting Temporal Variability. Journal of Geophysical Research: Atmospheres, 103(D17): 21943-21954. doi: 10.1029/98jd01358
    Guo, H., Wang, T., Simpson, I. J., et al., 2004. Source Contributions to Ambient VOCs and CO at a Rural Site in Eastern China. Atmospheric Environment, 38(27): 4551-4560. doi: 10.1016/j.atmosenv.2004.05.004
    Hao, J. M., Wang, L. T., Shen, M. J., et al., 2007. Air Quality Impacts of Power Plant Emissions in Beijing. Environmental Pollution, 147(2): 401-408. doi: 10.1016/j.envpol.2006.06.013
    Hong, S. M., Barbante, C., Boutron, C., et al., 2004. Atmospheric Heavy Metals in Tropical South America during the Past 22 000 Years Recorded in a High Altitude Ice Core from Sajama, Bolivia. Journal of Environmental Monitoring, 6(4): 322-326. doi: 10.1039/b314251e
    Hoornaert, S., Godoi, R. H. M., van Grieken, R., 2004. Elemental and Single Particle Aerosol Characterisation at a Background Station in Kazakhstan. Journal of Atmospheric Chemistry, 48(3): 301-315. doi: 10.1023/b:joch.0000044432.74476.b0
    Huang, K., Fu, J. S., Gao, Y., et al., 2014. Role of Sectoral and Multi-Pollutant Emission Control Strategies in Improving Atmospheric Visibility in the Yangtze River Delta, China. Environmental Pollution, 184: 426-434. doi: 10.1016/j.envpol.2013.09.029
    Hur Do, S., Soyol-Erdene, T. O., Hwang, H. J., et al., 2013. Climate-Related Variations in Atmospheric Sb and Tl in the EPICA Dome C Ice (East Antarctica) during the Past 800 000 Years. Global Biogeochemical Cycles, 27(3): 930-940. doi: 10.1002/gbc.20079
    Jaffe, D., Anderson, T., Covert, D., et al., 1999. Transport of Asian Air Pollution to North America. Geophysical Research Letters, 26(6): 711-714. doi: 10.1029/1999gl900100
    Jiang, Y. L., Zhuang, G. S., Wang, Q. Z., et al., 2014. Aerosol Oxalate and Its Implication to Haze Pollution in Shanghai, China. Chinese Science Bulletin, 59(2): 227-238. doi: 10.1007/s11434-013-0009-4
    Koçak, M., Nimmo, M., Kubilay, N., et al., 2004. Spatio-Temporal Aerosol Trace Metal Concentrations and Sources in the Levantine Basin of the Eastern Mediterranean. Atmospheric Environment, 38(14): 2133-2144. doi: 10.1016/j.atmosenv.2004.01.020
    Kubilay, N., Saydam, A. C., 1995. Trace Elements in Atmospheric Particulates over the Eastern Mediterranean; Concentrations, Sources, and Temporal Variability. Atmospheric Environment, 29(17): 2289-2300. doi: 10.1016/1352-2310(95)00101-4
    Lee, K., Hur Do, S., Hou, S. G., et al., 2008. Atmospheric Pollution for Trace Elements in the Remote High-Altitude Atmosphere in Central Asia as Recorded in Snow from Mt. Qomolangma (Everest) of the Himalayas. Science of the Total Environment, 404(1): 171-181. doi: 10.1016/j.scitotenv.2008.06.022
    Li, J., Zhuang, G. S., Huang, K., et al., 2008. Characteristics and Sources of Air-Borne Particulate in Urumqi, China, the Upstream Area of Asia Dust. Atmospheric Environment, 42(4): 776-787. doi: 10.1016/j.atmosenv.2007.09.062
    Li, Q., Song, J. P., Wang, E. R., et al., 2014. Economic Growth and Pollutant Emissions in China: A Spatial Econometric Analysis. Stochastic Environmental Research and Risk Assessment, 28(2): 429-442. doi: 10.1007/s00477-013-0762-6
    Lu, C., Deng, Q. H., Ou, C. Y., et al., 2013. Effects of Ambient Air Pollution on Allergic Rhinitis among Preschool Children in Changsha, China. Chinese Science Bulletin, 58(34): 4252-4258. doi: 10.1007/s11434-013-5725-2
    Lu, H., Zhu, L. Z., Chen, S. G., 2008. Pollution Level, Phase Distribution and Health Risk of Polycyclic Aromatic Hydrocarbons in Indoor Air at Public Places of Hangzhou, China. Environmental Pollution, 152(3): 569-575. doi: 10.1016/j.envpol.2007.07.005
    Mamtimin, B., Meixner, F. X., 2007. The Characteristics of Airpollution in the Semi-Arid City of Urumqi (NW China) and Its Relation to Climatological Process. Geophysical Research Abstracts, 9: 06537
    MEP (Ministry of Environmental Protection of the Peolie's Repubulic of China), GAQS (General Adminishtration of Quality Supervision, Inspection and Quantantine of the People's Republic of China), 2012. Ambient Air Quality Standard: GB 3095-2012. China Environmental Press, Beijing
    Nriagu, J. O., 1989. A Global Assessment of Natural Sources of Atmospheric Trace-Metals. Nature, 338(6210): 47-49. doi: 10.1038/338047a0
    Okuda, T., Katsuno, M., Naoi, D., et al., 2008. Trends in Hazardous Trace Metal Concentrations in Aerosols Collected in Beijing, China from 2001 to 2006. Chemosphere, 72: 917-924 doi: 10.1016/j.chemosphere.2008.03.033
    Olivier, S., Schwikowski, M., Brutsch, S., et al., 2003. Glaciochemical Investigation of an Ice Core from Belukha Glacier, Siberian Altai. Geophysical Research Letters, 30(19): 313-324. doi: 10.1029/2003gl018290
    Öztürk, F., Zararsız, A., Dutkiewicz, V. A., et al., 2012. Temporal Variations and Sources of Eastern Mediterranean Aerosols Based on a 9-Year Observation. Atmospheric Environment, 61: 463-475. doi: 10.1016/j.atmosenv.2012.07.051
    Pacyna, J. M., Pacyna, E. G., 2001. An Assessment of Global and Regional Emissions of Trace Metals to the Atmosphere from Anthropogenic Sources Worldwide. Environmental Reviews, 9(4): 269-298. doi: 10.1139/er-9-4-269
    Paoletti, L., De Berardis, B., Arrizza, L., et al., 2003. Seasonal Effects on the Physico-Chemical Characteristics of PM2.1 in Rome: A Study by SEM and XPS. Atmospheric Environment, 37(35): 4869-4879. doi: 10.1016/j.atmosenv.2003.08.031
    Pey, J., Alastuey, A., Querol, X., et al., 2010. Monitoring of Sources and Atmospheric Processes Controlling Air Quality in an Urban Mediterranean Environment. Atmospheric Environment, 44(38): 4879-4890. doi: 10.1016/j.atmosenv.2010.08.034
    Pósfai, M., Simonics, R., Li, J., et al., 2003. Individual Aerosol Particles from Biomass Burning in Southern Africa: 1. Compositions and Size Distributions of Carbonaceous Particles. Journal of Geophysical Research, 108(D13): 865-876. doi: 10.1029/2002jd002291
    Sexton, K., Westberg, H., 1984. Nonmethane Hydrocarbon Composition of Urban and Rural Atmospheres. Atmospheric Environment, 18(6): 1125-1132. doi: 10.1016/0004-6981(84)90144-6
    Shen, G. F., Yuan, S. Y., Xie, Y. N., et al., 2014. Ambient Levels and Temporal Variations of PM2.5 and PM10 at a Residential Site in the Mega-City, Nanjing, in the Western Yangtze River Delta, China. Journal of Environment Science and Health, Part A, 49(2): 171-178. doi: 10.1080/10934529.2013.838851
    Shi, G. T., Chen, Z. L., Xu, S. Y., et al., 2008. Potentially Toxic Metal Contamination of Urban Soils and Roadside Dust in Shanghai. China, Environmental Pollution, 156(2): 251-260. doi: 10.1016/j.envpol.2008.02.027
    Sun, J. M., Zhang, M. Y., Liu, T. S., 2001. Spatial and Temporal Characteristics of Dust Storms in China and Its Surrounding Regions, 1960-1999: Relations to Source Area and Climate. Journal of Geophysical Research, 106(D10): 10325-10333. doi: 10.1029/2000jd900665
    Tan, H. B., Yin, Y., Gu, X. S., et al., 2013. An Observational Study of the Hygroscopic Properties of Aerosols over the Pearl River Delta Region. Atmospheric Environment, 77: 817-826. doi: 10.1016/j.atmosenv.2013.05.049
    Wang, F. T., Wang, L., Kang, J., et al., 2011. Chemical Characteristics of Snow-Firn Pack in Altai Mountains and Its Environmental Significance. Journal of Earth Science, 22(4): 482-489. doi: 10.1007/s12583-011-0202-9
    Wang, Q., Bi, X. H., Wu, J. H., et al., 2013. Heavy Metals in Urban Ambient PM10 and Soil Background in Eight Cities around China. Environmental Monitoring and Assessment, 185(2): 1473-1482. doi: 10.1007/s10661-012-2646-5
    Wang, X. K., Manning, W., Feng, Z.W., et al., 2007. Ground-Level Ozone in China: Distribution and Effects on Crop Yields. Environmental Pollution, 147(2): 394-400. doi: 10.1016/j.envpol.2006.05.006
    Wedepohl, K. H., 1995. The Composition of the Continental-Crust. Geochimica et Cosmochimica Acta, 59(7): 1217-1232. doi: 10.1016/0016-7037(95)00038-2
    Wei, J. C., Guo, X. M., Marinova, D., et al., 2014. Industrial SO2 Pollution and Agricultural Losses in China: Evidence from Heavy Air Polluters. Journal of Cleaner Production, 64(1): 404-413. doi: 10.1016/j.jclepro.2013.10.027
    Wong, S. C., Li, X. D., Zhang, G., et al., 2002. Heavy Metals in Agricultural Soils of the Pearl River Delta, South China. Environmental Pollution, 119(1): 33-44. doi: 10.1016/s0269-7491(01)00325-6
    Wu, D. W., Yang, D. G., Mao, H. Y., et al., 2008. Structuring Recycle Economy of Advantageous Industries: A Case Study of Fukang City. Arid Land Geography, 31(5): 779-787 (in Chinese with English Abstract) http://www.cabdirect.org/abstracts/20113108122.html
    Wu, G. J., Xu, B. Q., Yao, T. D., et al., 2009. Heavy Metals in Aerosol Samples from the Eastern Pamirs Collected 2004-2006. Atmospheric Research, 93: 784-792. doi: 10.1016/j.atmosres.2009.03.011
    Xiao, R., Bai, J. H., Huang, L. B., et al., 2013. Distribution and Pollution, Toxicity and Risk Assessment of Heavy Metals in Sediments from Urban and Rural Rivers of the Pearl River Delta in Southern China. Ecotoxicology, 22(10): 1564-1575. doi: 10.1007/s10646-013-1142-1
    Yang, D. Z., Yu, H. Q., Ding, G. A., et al., 2003. An Analysis of Aerosols in the Lower-Leve Atmosphere over Beijing Northern Suburbs in Winter. Acta Meteorologica Sinica, 17: 117-128 (in Chinese with English Abstract) http://en.cnki.com.cn/Article_en/CJFDTOTAL-YYQX2002S1012.htm
    Yang, G., Xiao, L., Wang, G. C., et al., 2015. Geochronological, Geochemical and Petrogenesis of Bieluagaxi Granodioritic Pluton in Western Junggar. Earth Science--Journal of China University of Geosciences, 40(5): 810-823 (in Chinese with English Abstract) https://www.researchgate.net/publication/281690101_Geochronological_geochemical_and_petrogenesis_of_Bieluagaxi_granodioritic_pluton_in_western_Junggar
    Yin, W. Q., Wang, L., Li, R. R., et al., 2014. Personal Exposure Levels of PAHs in the General Population in Northern Rural Area of Jiangsu Province, China. Journal of Environment Science and Health, Part A: Toxic/Hazardous Substances and Environmental Engineering, 49(3): 281-286. doi: 10.1080/10934529.2014.846604
    Yue, W. S., Lia, X. L., Liu, J. F., et al., 2006. Characterization of PM2.5 in the Ambient Air of Shanghai City by Analyzing Individual Particles. Science of the Total Environment, 368(2/3): 916-925. doi: 10.1016/j.scitotenv.2006.03.043
    Zhang, D. J., Liu, X. Y., Wang, Y. H., et al., 2015. Sedimentary Evolution and Reservoir Characteristics of Carbonate Rocks since Late Miocene in Xisha Area of the South China Sea. Earth Science--Journal of China University of Geosciences, 40(4): 606-614 (in Chinese with English Abstract) doi: 10.3799/dqkx.2015.048
    Zhang, X. Y., Edwards, R., 2011. Anthropogenic Sulfate and Nitrate Signals in Snow from Bogda Glacier, Eastern Tianshan. Journal of Earth Science, 22(4): 490-502. doi: 10.1007/s12583-011-0196-3
    Zhao, S. H., Li, Z. Q., Zhou, P., 2011. Ion Chemistry and Individual Particle Analysis of Atmospheric Aerosols over Mt. Bogda of Eastern Tianshan Mountains, Central Asia, Environmental Monitoring and Assessment, 180(1/2/3/4): 409-426. doi: 10.1007/s10661-010-1796-6
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Figures(6)  / Tables(2)

    Article Metrics

    Article views(312) PDF downloads(1) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return