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Volume 32 Issue 4
Aug 2021
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Journal of Earth Science  > 2021  >  32(4): 887-900.
Zhen Qiu, Huifei Tao, Bin Lu, Zhenhong Chen, Songtao Wu, Hanlin Liu, Junli Qiu. Controlling Factors on Organic Matter Accumulation of Marine Shale across the Ordovician-Silurian Transition in South China: Constraints from Trace-Element Geochemistry. Journal of Earth Science, 2021, 32(4): 887-900. doi: 10.1007/s12583-020-1359-x
Citation: Zhen Qiu, Huifei Tao, Bin Lu, Zhenhong Chen, Songtao Wu, Hanlin Liu, Junli Qiu. Controlling Factors on Organic Matter Accumulation of Marine Shale across the Ordovician-Silurian Transition in South China: Constraints from Trace-Element Geochemistry. Journal of Earth Science, 2021, 32(4): 887-900. doi: 10.1007/s12583-020-1359-x
shu

Controlling Factors on Organic Matter Accumulation of Marine Shale across the Ordovician-Silurian Transition in South China: Constraints from Trace-Element Geochemistry

doi: 10.1007/s12583-020-1359-x
  • 1.

    Research Institute of Petroleum Exploration and Development, CNPC, Beijing 100083, China

  • 2.

    National Energy Shale Gas Research and Development(Experiment) Center, Langfang 065007, China

  • 3.

    Oil and Gas Research Center, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China

  • 4.

    Key Laboratory of Oil and Gas Reservoirs, CNPC, Beijing 100083, China

  • 5.

    National Energy Tight Oil and Gas R; D Center, Beijing 100083, China

  • 6.

    Institute of Oil and Gas, Peking University, Beijing 100871, China

More Information
  • Corresponding author: Huifei Tao, tophic3@yeah.net
  • Received Date: 08 Apr 2020
  • Accepted Date: 15 Jun 2020
  • Publish Date: 16 Aug 2021
    Abstract
  • In recent years, significant progress in shale gas exploration has been achieved in the Upper Ordovician (Wufeng Formation)-Lower Silurian (Longmaxi Formation) shales in the Upper Yangtze area, South China. Although many studies have been carried out on the Upper Ordovician-Lower Silurian shales, the controlling factors causing organic matter accumulation of these shales remain controversial. This study uses trace-element geochemistry and sedimentological methods to evaluate terrigenous input, redox conditions and primary productivity to explore the mechanisms of organic matter accumulation. The variation of terrigenous fraction elements (Al, Th and Sc) concentrations reflect a mixed influence of sea-level change and weathering. The sea-level of the Upper Yangtze Sea went through two cycles of transgression to regression during the Ordovician-Silurian transition. The Linxiang Formation, Kuanyinchiao Bed and the upper part of Longmaxi Formation developed during the periods of regression, whereas the Wufeng Formation and the lower part of the Longmaxi Formation developed during the periods of transgression. The paleo-productivity indexes of TOC content, ratios of Ba/Al and P/Al, and redox conditions proxies of Mo concentration, ratios of U/Th and V/Cr generally display similar variation patterns with respect to the sea-level changes. High TOC contents and Ba/Al and P/Al ratios indicate the paleo-productivity was high on the sea surface, as shown by relatively good positive correlations between Th vs. TOC, and Sc vs. TOC. This indicates that the paleo-productivity was controlled by the nutrients input through weathering. The good positive correlations between redox conditions indexes (U/Th and V/Cr ratios) with TOC content reflects reductive preservation conditions (anoxic to euxinic), thus implying they were an important controlling factor for organic matter accumulation. Nevertheless, redox conditions were closely associated with sea level change and organic matter decomposition. Therefore, the sea-level change and weathering were the primary controlling factors for organic matter enrichment across the Ordovician to Silurian transition.

     

    • Electronic Supplementary Materials: Supplementary materials (Tables S1–S3 and Figs. S1–S3) are available in the online version of this article at https://doi.org/10.1007/s12583-020-1359-x.
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